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The catalytic activity of bimetallic FeCoBEA zeolite catalysts in Fischer-Tropsch synthesis : the role of cobalt in framework position of dealuminated SiBEA zeolite
BEA zeolite
Fischer-Tropsch synthesis
cobalt catalysts
iron catalysts
bimetallic iron‑cobalt catalysts
Two series of BEA zeolite modified with transition metals (Co and Fe) with different metals loadings were obtained: the first one was prepared by classical sequential wet impregnation to obtain C-Fe
dc.abstract.en | Two series of BEA zeolite modified with transition metals (Co and Fe) with different metals loadings were obtained: the first one was prepared by classical sequential wet impregnation to obtain C-Fe$_{x}$Co$_{y}$AlBEA catalysts; the second one was obtained by a two-step postsynthesis method to design C-Fe$_{x}$Co$_{y}$SiBEA catalysts. The catalytic activity of both series of FeCoBEA zeolite catalysts was determined by the FTS process. These bimetallic catalysts appear to combine the advantages of monometallic cobalt catalysts (lower selectivity towards CO$_{2}$ than for monometallic iron catalysts) and iron catalysts (lower selectivity towards CH$_{4}$ than for monometallic cobalt catalysts), while minimizing their disadvantages, such as the large amount of carbon deposition. | |
dc.affiliation | Wydział Fizyki, Astronomii i Informatyki Stosowanej : Instytut Fizyki im. Mariana Smoluchowskiego | |
dc.contributor.author | Chałupka-Śpiewak, Karolina A. | |
dc.contributor.author | Gurgul, Jacek | |
dc.contributor.author | Grams, Jacek | |
dc.contributor.author | Mierczyński, Paweł | |
dc.contributor.author | Maniukiewicz, Waldemar | |
dc.contributor.author | Szynkowska-Jóźwik, Małgorzata I. | |
dc.contributor.author | Łątka, Kazimierz - 100050 | |
dc.contributor.author | Rynkowski, Jacek | |
dc.contributor.author | Dźwigaj, Stanisław | |
dc.date.accessioned | 2025-02-21T15:37:14Z | |
dc.date.available | 2025-02-21T15:37:14Z | |
dc.date.createdat | 2025-02-21T13:55:28Z | en |
dc.date.issued | 2024 | |
dc.date.openaccess | 0 | |
dc.description.accesstime | w momencie opublikowania | |
dc.description.version | ostateczna wersja wydawcy | |
dc.description.volume | 192 | |
dc.identifier.articleid | 206935 | |
dc.identifier.doi | 10.1016/j.apcato.2024.206935 | |
dc.identifier.eissn | 2950-6484 | |
dc.identifier.issn | 2950-6492 | |
dc.identifier.uri | https://ruj.uj.edu.pl/handle/item/549193 | |
dc.language | eng | |
dc.language.container | eng | |
dc.rights | Udzielam licencji. Uznanie autorstwa - Użycie niekomercyjne 4.0 Międzynarodowa | |
dc.rights.licence | CC-BY-NC | |
dc.rights.uri | http://creativecommons.org/licenses/by-nc/4.0/legalcode.pl | |
dc.share.type | otwarte czasopismo | |
dc.subject.en | BEA zeolite | |
dc.subject.en | Fischer-Tropsch synthesis | |
dc.subject.en | cobalt catalysts | |
dc.subject.en | iron catalysts | |
dc.subject.en | bimetallic iron‑cobalt catalysts | |
dc.subtype | Article | |
dc.title | The catalytic activity of bimetallic FeCoBEA zeolite catalysts in Fischer-Tropsch synthesis : the role of cobalt in framework position of dealuminated SiBEA zeolite | |
dc.title.journal | Applied Catalysis O: Open | |
dc.type | JournalArticle | |
dspace.entity.type | Publication | en |