TbRhSn and DyRhSn - Detailed magnetic and ^{119}Sn Mössbauer spectroscopic studies

2014
journal article
article
6
dc.abstract.enThe results of magnetic studies and Mössbauer spectroscopic investigations are reported for the stannides TbRhSn and DyRhSn crystallizing in the hexagonal ZrNiAl-type structure. The polycrystalline samples of these ternary intermetallics were synthesized by arc melting from metallic precursors. Detailed ^{119}Sn Mössbauer spectroscopic studies are used to investigate the hyperfine interactions and their temperature evolutions at places occupied by the diamagnetic tin nuclei. Magnetic properties of DyRhSn and TbRhSn were studied by AC/DC magnetometry in a wide temperature range. The results show that both compounds are magnetically ordered at low temperatures. DyRhSn is a non-collinear antiferromagnet with the Néel temperature T_{N} = 7.5 K, whereas TbRhSn undergoes a transition from a paramagnetic to an antiferromagnetic state at T_{N} = 20.2 K. An additional transition at T_{SR} = 10.3 K is detected for TbRhSn which corresponds to some changes in the magnetic moments ordering. The role of the magnetostriction effect in the evolution of the hyperfine parameters and its influence on the observed TbRhSn Mössbauer spectra is discussed. Triangular-like antiferromagnetic arrangements with rare-earth magnetic moments lying in the hexagonal plane are proposed for both compounds at very low temperatures.pl
dc.affiliationWydział Fizyki, Astronomii i Informatyki Stosowanej : Instytut Fizyki im. Mariana Smoluchowskiegopl
dc.contributor.authorGurgul, Jacekpl
dc.contributor.authorŁątka, Kazimierz - 100050 pl
dc.contributor.authorPacyna, Andrzej W.pl
dc.contributor.authorPeter, Sebastian C.pl
dc.contributor.authorPöttgen, Rainerpl
dc.date.accessioned2015-02-27T08:48:26Z
dc.date.available2015-02-27T08:48:26Z
dc.date.issued2014pl
dc.description.physical56-64pl
dc.description.publication0,5pl
dc.description.volume46pl
dc.identifier.doi10.1016/j.intermet.2013.10.020pl
dc.identifier.eissn1879-0216pl
dc.identifier.issn0966-9795pl
dc.identifier.urihttp://ruj.uj.edu.pl/xmlui/handle/item/3361
dc.languageengpl
dc.language.containerengpl
dc.rightsDodaję tylko opis bibliograficzny*
dc.rights.licenceBez licencji otwartego dostępu
dc.rights.uri*
dc.subject.enrare-earth intermetallicspl
dc.subject.enmagnetic propertiespl
dc.subject.enspectroscopic methodspl
dc.subtypeArticlepl
dc.titleTbRhSn and DyRhSn - Detailed magnetic and ^{119}Sn Mössbauer spectroscopic studiespl
dc.title.journalIntermetallicspl
dc.typeJournalArticlepl
dspace.entity.typePublication
dc.abstract.enpl
The results of magnetic studies and Mössbauer spectroscopic investigations are reported for the stannides TbRhSn and DyRhSn crystallizing in the hexagonal ZrNiAl-type structure. The polycrystalline samples of these ternary intermetallics were synthesized by arc melting from metallic precursors. Detailed ^{119}Sn Mössbauer spectroscopic studies are used to investigate the hyperfine interactions and their temperature evolutions at places occupied by the diamagnetic tin nuclei. Magnetic properties of DyRhSn and TbRhSn were studied by AC/DC magnetometry in a wide temperature range. The results show that both compounds are magnetically ordered at low temperatures. DyRhSn is a non-collinear antiferromagnet with the Néel temperature T_{N} = 7.5 K, whereas TbRhSn undergoes a transition from a paramagnetic to an antiferromagnetic state at T_{N} = 20.2 K. An additional transition at T_{SR} = 10.3 K is detected for TbRhSn which corresponds to some changes in the magnetic moments ordering. The role of the magnetostriction effect in the evolution of the hyperfine parameters and its influence on the observed TbRhSn Mössbauer spectra is discussed. Triangular-like antiferromagnetic arrangements with rare-earth magnetic moments lying in the hexagonal plane are proposed for both compounds at very low temperatures.
dc.affiliationpl
Wydział Fizyki, Astronomii i Informatyki Stosowanej : Instytut Fizyki im. Mariana Smoluchowskiego
dc.contributor.authorpl
Gurgul, Jacek
dc.contributor.authorpl
Łątka, Kazimierz - 100050
dc.contributor.authorpl
Pacyna, Andrzej W.
dc.contributor.authorpl
Peter, Sebastian C.
dc.contributor.authorpl
Pöttgen, Rainer
dc.date.accessioned
2015-02-27T08:48:26Z
dc.date.available
2015-02-27T08:48:26Z
dc.date.issuedpl
2014
dc.description.physicalpl
56-64
dc.description.publicationpl
0,5
dc.description.volumepl
46
dc.identifier.doipl
10.1016/j.intermet.2013.10.020
dc.identifier.eissnpl
1879-0216
dc.identifier.issnpl
0966-9795
dc.identifier.uri
http://ruj.uj.edu.pl/xmlui/handle/item/3361
dc.languagepl
eng
dc.language.containerpl
eng
dc.rights*
Dodaję tylko opis bibliograficzny
dc.rights.licence
Bez licencji otwartego dostępu
dc.rights.uri*
dc.subject.enpl
rare-earth intermetallics
dc.subject.enpl
magnetic properties
dc.subject.enpl
spectroscopic methods
dc.subtypepl
Article
dc.titlepl
TbRhSn and DyRhSn - Detailed magnetic and ^{119}Sn Mössbauer spectroscopic studies
dc.title.journalpl
Intermetallics
dc.typepl
JournalArticle
dspace.entity.type
Publication
Affiliations

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