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Structure of the indium-rich InSb(001) surface
The indium-rich InSb(001) surface, that shows the c(8×2) reconstruction at room temperature and a partially disordered phase at 77 K (the low temperature or LT phase), is studied experimentally by means of scanning probe microscopies, low-energy electron diffraction, and angle-resolved photoelectron spectroscopy (ARPES), as well as theoretically, using the density-functional theory (DFT). The experimental studies are done both at room temperature and at cryogenic temperatures. No metallic surface bands are found using ARPES, consequently the idea of charge-density waves as a possible explanation of the LT phase suggested previously by Goryl et al. [Surf. Sci. 601, 3605 (2007)] is discarded. On the other hand it is shown that an essential core of the surface structure is described by the so-called ζ model which has the c(8×2) symmetry. However, on top of this basic structure there are additional not fully occupied indium-atom rows. Vacancies/atoms in these rows rapidly fluctuate at room temperature while, upon cooling down, they stabilize to form a sublattice also of c(8×2) symmetry. Furthermore, this sublattice has shifted mirror symmetry axes (relating to those of the underlying ζ lattice) therefore the surface symmetry is lowered from c2mm to p2 and structural domains are formed. This occurs with no significant core ζ lattice distortions but dense domain borders lead to significant disorder in the top atomic layer. DFT calculations confirm that the postulated ζ-like structure with additional 50% occupied indium-atom rows is stable on the InSb (001) surface. Calculated, in the Tersoff-Hammann approximation, scanning tunneling microscopy (STM) images of the relaxed surface structure agree well with experimental STM images.
dc.abstract.en | The indium-rich InSb(001) surface, that shows the c(8×2) reconstruction at room temperature and a partially disordered phase at 77 K (the low temperature or LT phase), is studied experimentally by means of scanning probe microscopies, low-energy electron diffraction, and angle-resolved photoelectron spectroscopy (ARPES), as well as theoretically, using the density-functional theory (DFT). The experimental studies are done both at room temperature and at cryogenic temperatures. No metallic surface bands are found using ARPES, consequently the idea of charge-density waves as a possible explanation of the LT phase suggested previously by Goryl et al. [Surf. Sci. 601, 3605 (2007)] is discarded. On the other hand it is shown that an essential core of the surface structure is described by the so-called ζ model which has the c(8×2) symmetry. However, on top of this basic structure there are additional not fully occupied indium-atom rows. Vacancies/atoms in these rows rapidly fluctuate at room temperature while, upon cooling down, they stabilize to form a sublattice also of c(8×2) symmetry. Furthermore, this sublattice has shifted mirror symmetry axes (relating to those of the underlying ζ lattice) therefore the surface symmetry is lowered from c2mm to p2 and structural domains are formed. This occurs with no significant core ζ lattice distortions but dense domain borders lead to significant disorder in the top atomic layer. DFT calculations confirm that the postulated ζ-like structure with additional 50% occupied indium-atom rows is stable on the InSb (001) surface. Calculated, in the Tersoff-Hammann approximation, scanning tunneling microscopy (STM) images of the relaxed surface structure agree well with experimental STM images. | pl |
dc.affiliation | Wydział Fizyki, Astronomii i Informatyki Stosowanej : Instytut Fizyki im. Mariana Smoluchowskiego | pl |
dc.contributor.author | Goryl, Grzegorz - 102886 | pl |
dc.contributor.author | Toton, Dawid - 106941 | pl |
dc.contributor.author | Tomaszewska, Natalia | pl |
dc.contributor.author | Prauzner-Bechcicki, Jakub - 160675 | pl |
dc.contributor.author | Walczak, Łukasz - 185657 | pl |
dc.contributor.author | Tejeda, Antonio | pl |
dc.contributor.author | Taleb-Ibrahimi, Amina | pl |
dc.contributor.author | Kantorovich, Lev | pl |
dc.contributor.author | Michel, Enrique García | pl |
dc.contributor.author | Kołodziej, Jacek - 129019 | pl |
dc.date.accessioned | 2015-01-26T09:39:45Z | |
dc.date.available | 2015-01-26T09:39:45Z | |
dc.date.issued | 2010 | pl |
dc.description.admin | [AB] Tomaszewska, Natalia 50000139 | |
dc.description.number | 16 | pl |
dc.description.publication | 1 | pl |
dc.description.volume | 82 | pl |
dc.identifier.articleid | 165311 | pl |
dc.identifier.doi | 10.1103/PhysRevB.82.165311 | pl |
dc.identifier.eissn | 1550-235X | pl |
dc.identifier.eissn | 1538-4489 | pl |
dc.identifier.issn | 1098-0121 | pl |
dc.identifier.uri | http://ruj.uj.edu.pl/xmlui/handle/item/2732 | |
dc.language | eng | pl |
dc.language.container | eng | pl |
dc.rights | Dodaję tylko opis bibliograficzny | * |
dc.rights.uri | * | |
dc.subtype | Article | pl |
dc.title | Structure of the indium-rich InSb(001) surface | pl |
dc.title.journal | Physical Review. B, Condensed Matter and Materials Physics | pl |
dc.type | JournalArticle | pl |
dspace.entity.type | Publication |