Structure of the indium-rich InSb(001) surface

2010
journal article
article
10
dc.abstract.enThe indium-rich InSb(001) surface, that shows the c(8×2) reconstruction at room temperature and a partially disordered phase at 77 K (the low temperature or LT phase), is studied experimentally by means of scanning probe microscopies, low-energy electron diffraction, and angle-resolved photoelectron spectroscopy (ARPES), as well as theoretically, using the density-functional theory (DFT). The experimental studies are done both at room temperature and at cryogenic temperatures. No metallic surface bands are found using ARPES, consequently the idea of charge-density waves as a possible explanation of the LT phase suggested previously by Goryl et al. [Surf. Sci. 601, 3605 (2007)] is discarded. On the other hand it is shown that an essential core of the surface structure is described by the so-called ζ model which has the c(8×2) symmetry. However, on top of this basic structure there are additional not fully occupied indium-atom rows. Vacancies/atoms in these rows rapidly fluctuate at room temperature while, upon cooling down, they stabilize to form a sublattice also of c(8×2) symmetry. Furthermore, this sublattice has shifted mirror symmetry axes (relating to those of the underlying ζ lattice) therefore the surface symmetry is lowered from c2mm to p2 and structural domains are formed. This occurs with no significant core ζ lattice distortions but dense domain borders lead to significant disorder in the top atomic layer. DFT calculations confirm that the postulated ζ-like structure with additional 50% occupied indium-atom rows is stable on the InSb (001) surface. Calculated, in the Tersoff-Hammann approximation, scanning tunneling microscopy (STM) images of the relaxed surface structure agree well with experimental STM images.pl
dc.affiliationWydział Fizyki, Astronomii i Informatyki Stosowanej : Instytut Fizyki im. Mariana Smoluchowskiegopl
dc.contributor.authorGoryl, Grzegorz - 102886 pl
dc.contributor.authorToton, Dawid - 106941 pl
dc.contributor.authorTomaszewska, Nataliapl
dc.contributor.authorPrauzner-Bechcicki, Jakub - 160675 pl
dc.contributor.authorWalczak, Łukasz - 185657 pl
dc.contributor.authorTejeda, Antoniopl
dc.contributor.authorTaleb-Ibrahimi, Aminapl
dc.contributor.authorKantorovich, Levpl
dc.contributor.authorMichel, Enrique Garcíapl
dc.contributor.authorKołodziej, Jacek - 129019 pl
dc.date.accessioned2015-01-26T09:39:45Z
dc.date.available2015-01-26T09:39:45Z
dc.date.issued2010pl
dc.description.admin[AB] Tomaszewska, Natalia 50000139
dc.description.number16pl
dc.description.publication1pl
dc.description.volume82pl
dc.identifier.articleid165311pl
dc.identifier.doi10.1103/PhysRevB.82.165311pl
dc.identifier.eissn1550-235Xpl
dc.identifier.eissn1538-4489pl
dc.identifier.issn1098-0121pl
dc.identifier.urihttp://ruj.uj.edu.pl/xmlui/handle/item/2732
dc.languageengpl
dc.language.containerengpl
dc.rightsDodaję tylko opis bibliograficzny*
dc.rights.uri*
dc.subtypeArticlepl
dc.titleStructure of the indium-rich InSb(001) surfacepl
dc.title.journalPhysical Review. B, Condensed Matter and Materials Physicspl
dc.typeJournalArticlepl
dspace.entity.typePublication
dc.abstract.enpl
The indium-rich InSb(001) surface, that shows the c(8×2) reconstruction at room temperature and a partially disordered phase at 77 K (the low temperature or LT phase), is studied experimentally by means of scanning probe microscopies, low-energy electron diffraction, and angle-resolved photoelectron spectroscopy (ARPES), as well as theoretically, using the density-functional theory (DFT). The experimental studies are done both at room temperature and at cryogenic temperatures. No metallic surface bands are found using ARPES, consequently the idea of charge-density waves as a possible explanation of the LT phase suggested previously by Goryl et al. [Surf. Sci. 601, 3605 (2007)] is discarded. On the other hand it is shown that an essential core of the surface structure is described by the so-called ζ model which has the c(8×2) symmetry. However, on top of this basic structure there are additional not fully occupied indium-atom rows. Vacancies/atoms in these rows rapidly fluctuate at room temperature while, upon cooling down, they stabilize to form a sublattice also of c(8×2) symmetry. Furthermore, this sublattice has shifted mirror symmetry axes (relating to those of the underlying ζ lattice) therefore the surface symmetry is lowered from c2mm to p2 and structural domains are formed. This occurs with no significant core ζ lattice distortions but dense domain borders lead to significant disorder in the top atomic layer. DFT calculations confirm that the postulated ζ-like structure with additional 50% occupied indium-atom rows is stable on the InSb (001) surface. Calculated, in the Tersoff-Hammann approximation, scanning tunneling microscopy (STM) images of the relaxed surface structure agree well with experimental STM images.
dc.affiliationpl
Wydział Fizyki, Astronomii i Informatyki Stosowanej : Instytut Fizyki im. Mariana Smoluchowskiego
dc.contributor.authorpl
Goryl, Grzegorz - 102886
dc.contributor.authorpl
Toton, Dawid - 106941
dc.contributor.authorpl
Tomaszewska, Natalia
dc.contributor.authorpl
Prauzner-Bechcicki, Jakub - 160675
dc.contributor.authorpl
Walczak, Łukasz - 185657
dc.contributor.authorpl
Tejeda, Antonio
dc.contributor.authorpl
Taleb-Ibrahimi, Amina
dc.contributor.authorpl
Kantorovich, Lev
dc.contributor.authorpl
Michel, Enrique García
dc.contributor.authorpl
Kołodziej, Jacek - 129019
dc.date.accessioned
2015-01-26T09:39:45Z
dc.date.available
2015-01-26T09:39:45Z
dc.date.issuedpl
2010
dc.description.admin
[AB] Tomaszewska, Natalia 50000139
dc.description.numberpl
16
dc.description.publicationpl
1
dc.description.volumepl
82
dc.identifier.articleidpl
165311
dc.identifier.doipl
10.1103/PhysRevB.82.165311
dc.identifier.eissnpl
1550-235X
dc.identifier.eissnpl
1538-4489
dc.identifier.issnpl
1098-0121
dc.identifier.uri
http://ruj.uj.edu.pl/xmlui/handle/item/2732
dc.languagepl
eng
dc.language.containerpl
eng
dc.rights*
Dodaję tylko opis bibliograficzny
dc.rights.uri*
dc.subtypepl
Article
dc.titlepl
Structure of the indium-rich InSb(001) surface
dc.title.journalpl
Physical Review. B, Condensed Matter and Materials Physics
dc.typepl
JournalArticle
dspace.entity.type
Publication
Affiliations

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